Carrier confinement and bond softening in photoexcited bismuth films
نویسندگان
چکیده
Article is made available in accordance with the publisher's policy and may be subject to US copyright law. Please refer to the publisher's site for terms of use. The MIT Faculty has made this article openly available. Please share how this access benefits you. Your story matters.
منابع مشابه
Electron cooling and debye-waller effect in photoexcited bismuth.
By means of first principles calculations, we compute the effective electron-phonon coupling constant G(0) governing the electron cooling in photoexcited bismuth. G(0) strongly increases as a function of electron temperature, which can be traced back to the semimetallic nature of bismuth. We also use a thermodynamical model to compute the time evolution of both electron and lattice temperatures...
متن کاملPhotoexcited Carrier Lifetime and Refractive Nonlinearity in Direct and Indirect Band Gap Crystals on the Z-Scan Technique
The Photoexcited carrier lifetime (τ) and peak to valley transmission difference (ΔTp-v) in direct and indirect band gap crystals has been investigated by the use of single beam open and closed aperture z-scan technique using frequency doubled Nd:YAG laser. The peak to valley transmission difference (ΔTp-v) is found to be of the order of 10-2 in case of direct band gap crystals and of the order...
متن کاملProving Nontrivial Topology of Pure Bismuth by Quantum Confinement.
The topology of pure Bi is controversial because of its very small (∼10 meV) band gap. Here we perform high-resolution angle-resolved photoelectron spectroscopy measurements systematically on 14-202 bilayer Bi films. Using high-quality films, we succeed in observing quantized bulk bands with energy separations down to ∼10 meV. Detailed analyses on the phase shift of the confined wave function...
متن کاملPhotoexcited carrier relaxation dynamics in pentacene probed by ultrafast optical spectroscopy Influence of morphology on relaxation processes
We present a comparative study of ultrafast photoexcited state relaxation in pentacene single crystals and in pure and C60-doped pentacene films using optical pump-probe spectroscopy. The photoinduced absorption spectra in pentacene crystals is consistent with a dominant singlet–triplet fission decay channel for above-gap excitation. This decay channel is suppressed in thin films and even furth...
متن کاملUltrafast bond softening in bismuth: mapping a solid's interatomic potential with X-rays.
Intense femtosecond laser excitation can produce transient states of matter that would otherwise be inaccessible to laboratory investigation. At high excitation densities, the interatomic forces that bind solids and determine many of their properties can be substantially altered. Here, we present the detailed mapping of the carrier density-dependent interatomic potential of bismuth approaching ...
متن کاملذخیره در منابع من
با ذخیره ی این منبع در منابع من، دسترسی به آن را برای استفاده های بعدی آسان تر کنید
عنوان ژورنال:
دوره شماره
صفحات -
تاریخ انتشار 2015